Introduction¶
Set up a clean working directory and pull the example YAML:
$ mkdir my_dgeba_pacm
$ cd my_dgeba_pacm
$ htpolynet fetch-example 3
Fetched 3-pacm-dgeba-epoxy-thermoset.yaml (run with: htpolynet run 3-pacm-dgeba-epoxy-thermoset.yaml)
$ ls
3-pacm-dgeba-epoxy-thermoset.yaml
Self-contained YAML as in the earlier examples — both monomers are generated from SMILES with atom-mapping tokens at the start of the run.
What’s chemically new here is the epoxy + amine step-growth mechanism:
A primary amine (
-NH₂) opens an epoxide ring (C–O–C) to form a secondary amine and a pendant hydroxyl. The amine donates one H to the oxirane oxygen.The resulting secondary amine can react again with another epoxide, forming a tertiary amine. This second reaction is typically slower, which we encode with a per-reaction
probabilityin the YAML.Each PACM molecule can therefore tether up to four DGEBAs through its two nitrogens; each DGEBA can tether up to two amines through its two reactive carbons.
In the active form supplied to htpolynet, both oxiranes on DGEBA are
already “opened” into a primary alcohol + sacrificial methyl
configuration, so each reactive carbon carries a sacrificial H that gets
removed when a new C–N bond forms. The monomer page
walks through this in detail.